Date of Award

2024-12-01

Degree Name

Master of Science

Department

Mechanical Engineering

Advisor(s)

Evgeny Shafirovich

Abstract

Hydrogen as a fuel provides several benefits over the use of fossil fuels; however, one challenge in utilizing hydrogen as an energy carrier revolves around its storage. Achieving sufficient volumetric hydrogen density in a storage solution will facilitate hydrogenâ??s adoption for use in both stationary and mobile applications. Solid-state hydrogen storage provides a promising pathway to solving this problem. However, the hydrogenation of these materials is characterized by slow kinetics and extreme thermodynamic conditions. Magnesium borohydride (Mg(BH4)2) is a promising material in hydrogen storage due to its reversible properties and a theoretical hydrogen capacity of 14.9 wt.%. To synthesize this material, combustion synthesis of magnesium borides (MgBx) has been implemented with the aim to further lower thermodynamic requirements for direct hydrogenation. A drawback of this process is the potential formation of oxide contaminants, which decrease hydrogenation/dehydrogenation and recyclability performance. The present work focuses on identifying parameters useful for reducing contamination and evaluating potential pathways to the purification of magnesium borides with the goal of improving their quality.

Language

en

Provenance

Recieved from ProQuest

File Size

56 p.

File Format

application/pdf

Rights Holder

Miguel Joaquin Camarena

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